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While I think a lot of factors can figure in whether a tie can be knotted in this way, I suspect the lining is a big factor. Perhaps there's something more subtle in this knot that I'm not seeing, but I can usually get this effect by pulling the back blade out a bit when I cinch the knot, regardless of the tie. I don't usually do this, though. Maybe if the tie is a bit on the narrow side for the collar, but it otherwise feels a little iGent to me, at least when done in a bit more flamboyant way (the above is ok).
Why not think of it just as a coarsely woven textured tie with a very dry hand? Functionally, I tend to think of grossas as a close, more refined cousin of knits. The mottled effect just pushes it more in the casual direction.
I picked up a Drake's along these lines. It's very coarse in feel and I think will go quite nicely with tweed. So I say, go for it.